Linear dichroism in molecular resonant inelastic x-ray scattering
Polarization-dependent resonant inelastic x-ray scattering (RIXS) is shown to be a new probe of molecular-field effects on molecular electronic structure. Combining experiment and theory, linear dichroism in Cl 2p RIXS following Cl 1s excitation in HCl, Cl2, and CF3Cl is ascribed to molecular-field effects, indicating polarized-RIXS provides a direct probe of spin-orbit-state populations generally applicable to all molecules.
Analytical Chemistry | Atomic, Molecular and Optical Physics | Biological and Chemical Physics | Physical Chemistry
Use Find in Your Library, contact the author, or use interlibrary loan to garner a copy of the article. Publisher copyright policy allows author to archive post-print (author’s final manuscript). When post-print is available or publisher policy changes, the article will be deposited
Lindle, D. W.,
Stolte, W. C.,
Linear dichroism in molecular resonant inelastic x-ray scattering.
Journal of Physics: Conference Series, 194(2),