Linear Dichroism in Molecular Resonant Inelastic X-ray Scattering
Journal of Physics: Conference Series
First page number:
Polarization-dependent resonant inelastic x-ray scattering (RIXS) is shown to be a new probe of molecular-field effects on molecular electronic structure. Combining experiment and theory, linear dichroism in Cl 2p RIXS following Cl 1s excitation in HCl, Cl2, and CF3Cl is ascribed to molecular-field effects, indicating polarized-RIXS provides a direct probe of spin-orbit-state populations generally applicable to all molecules.
Atomic orbitals; Chloride compounds; Electron configuration; Linear dichroism
Analytical Chemistry | Atomic, Molecular and Optical Physics | Biological and Chemical Physics | Physical Chemistry
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Lindle, D. W.,
Stolte, W. C.,
Linear Dichroism in Molecular Resonant Inelastic X-ray Scattering.
Journal of Physics: Conference Series, 194(2),