Atmospheric Deposition of Particles at a Sensitive Alpine Lake: Size-Segregated Daily and Annual Fluxes From Passive Sampling Techniques
Document Type
Article
Publication Date
1-1-2017
Publication Title
Science of the Total Environment
Volume
579
First page number:
1736
Last page number:
1744
Abstract
Lake Tahoe, a North American alpine lake long appreciated for its clear water and geographic setting, has experienced a trend of declining water clarity due to increasing nutrient and particle inputs. Contributions from atmospheric deposition of particulate matter (PM) could be important, yet they are inadequately quantified. This study established a yearlong deposition monitoring network in the northern Lake Tahoe Basin. Dry deposition was quantified on surrogate surfaces while wet deposition was based on particles suspended in precipitation at 24-hour resolution. The particle size ranges by these passive techniques were 1–64 μm and 0.5–20 μm in diameter for dry and wet deposition, respectively. Dry deposition of submicrometer (0.5–1 μm) particles was also estimated by extrapolation of a lognormal size distribution. Higher daily number deposition fluxes (NDFdry and NDFwet) were found at a near-shore site, confirming substantial impacts of commercial and tourist activities. The two more isolated sites indicated a uniform regional background. On average, daily NDFdry is about one order of magnitude lower than daily NDFwet. Dry deposition velocities increased rapidly with particle size, as evidenced by collocated measurements of NDFdry and ambient particle number concentrations, though it seems less so for wet deposition due to different scavenging mechanisms. Despite fewer “wet” days than “dry” days during the monitoring period, wet processes dominated seasonal particle deposition, particularly in winter and spring when most precipitation occurred. Adopting sediment (insoluble, inorganic) particle fraction estimates from the literature, this study reports an annual particle flux of 2.9–5.2 × 1010 # m− 2 yr− 1 for sediment particles with 1–20 μm diameter and 6.1–11 × 1010 # m− 2 yr− 1 for those with 0.5–20 μm diameter. Implications of these findings to the current knowledge of atmospheric deposition in the Lake Tahoe Total Maximum Daily Load (TMDL) are discussed. © 2016 Elsevier B.V.
Language
english
Repository Citation
Tai, A. Y.,
Chen, L. A.,
Wang, X.,
Chow, J. C.,
Watson, J. G.
(2017).
Atmospheric Deposition of Particles at a Sensitive Alpine Lake: Size-Segregated Daily and Annual Fluxes From Passive Sampling Techniques.
Science of the Total Environment, 579
1736-1744.
http://dx.doi.org/10.1016/j.scitotenv.2016.11.117